Solvent effects in the nonlinear optical properties using the Voigt function
Nonlinear optical properties of a two-level molecular system immersed in a thermal bath have been studied in the present work. Solvent effects were explicitly considered by modeling the non-radiative interaction with the solute as a random variable. The innovation of this treatment is that it allows...
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oai:localhost:28000-38262017-11-01T18:15:33Z Solvent effects in the nonlinear optical properties using the Voigt function Paz Rojas, Jos? Luis PERMANENT DIPOLE MOMENTS ROTATING WAVE APPROXIMATION SOLVENT EFFECTS Nonlinear optical properties of a two-level molecular system immersed in a thermal bath have been studied in the present work. Solvent effects were explicitly considered by modeling the non-radiative interaction with the solute as a random variable. The innovation of this treatment is that it allows us to take into account the environment, inducing quantum effects not considered by classical treatment. The major contribution of the methodology proposed in this work, is the implementation of an approximant to the Voigt function as a probability distribution, because it allow us to cover a wider range of possible interactions among the solvent and the molecular system by simple changing the parameters ?L?L and ?G?G, associated to the variances of the Lorentzian and Gaussian distributions, respectively. http://www.worldscientific.com/doi/abs/10.1142/S0218863516500168 2017-04-12T17:49:42Z 2017-04-12T17:49:42Z 2016 article Paz, Jos? Luis. et al. (2016). Solvent effects in the nonlinear optical properties using the Voigt function. Journal of Nonlinear Optical Physics & Materials. Vol. 25, No. 02. pp.1-14 http://repositorio.educacionsuperior.gob.ec/handle/28000/3826 DOI:10.1142/S0218863516500168 closedAccess http://creativecommons.org/licenses/by-nc-sa/3.0/ec/ pp.1-14. |
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PERMANENT DIPOLE MOMENTS ROTATING WAVE APPROXIMATION SOLVENT EFFECTS |
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PERMANENT DIPOLE MOMENTS ROTATING WAVE APPROXIMATION SOLVENT EFFECTS Paz Rojas, Jos? Luis Solvent effects in the nonlinear optical properties using the Voigt function |
description |
Nonlinear optical properties of a two-level molecular system immersed in a thermal bath have been studied in the present work. Solvent effects were explicitly considered by modeling the non-radiative interaction with the solute as a random variable. The innovation of this treatment is that it allows us to take into account the environment, inducing quantum effects not considered by classical treatment. The major contribution of the methodology proposed in this work, is the implementation of an approximant to the Voigt function as a probability distribution, because it allow us to cover a wider range of possible interactions among the solvent and the molecular system by simple changing the parameters ?L?L and ?G?G, associated to the variances of the Lorentzian and Gaussian distributions, respectively. |
author |
Paz Rojas, Jos? Luis |
author_facet |
Paz Rojas, Jos? Luis |
author_sort |
Paz Rojas, Jos? Luis |
title |
Solvent effects in the nonlinear optical properties using the Voigt function |
title_short |
Solvent effects in the nonlinear optical properties using the Voigt function |
title_full |
Solvent effects in the nonlinear optical properties using the Voigt function |
title_fullStr |
Solvent effects in the nonlinear optical properties using the Voigt function |
title_full_unstemmed |
Solvent effects in the nonlinear optical properties using the Voigt function |
title_sort |
solvent effects in the nonlinear optical properties using the voigt function |
publishDate |
2017 |
url |
http://repositorio.educacionsuperior.gob.ec/handle/28000/3826 |
_version_ |
1634995194250133504 |
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11,871979 |